The famous actress came very close to being part of the fourth Spider-Man movie that never happened, as the daughter of The Vulture.
Sam Raimi wanted to invite Angelina Jolie and Anne Hathaway to the 4th Spider-Man movie, and the main villain was to be Vulture
Spider-Man / What Could Have Been - TV Tropes
Photos of Vulture's costume for Sam Raimi's cancelled Spider-Man 4 revealed, Entertainment News - AsiaOne
Spider-Man 4: Angelina Jolie was to appear in the film as the Vulture's daughter
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Angelina Jolie Almost Joined Marvel Long Before Eternals As a Villain!
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Original Spider-Man 4 canceled casting plans revealed - Dexerto
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Spider-Man: No Way Home' Poster Hints at Multiple Villains